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Medicinal Products Incorporating Bound Organosulfur Groups

por Tiffany Mott (2019-11-21)


Medicinal Products Incorporating Bound Organosulfur Groups
Abstrac
Nutraceutical and dietary supplement formulations for delivering bioavailable thiols to a host, comprising certain organosulfur radicals, such as the allyl mercapto radical, bound to larger molecules such as proteins, resulting in the formation in the host's body of various allium-related compounds such as allicin. The formulations are produced by treating an ingestible material comprising a cysteine-containing protein with a thiol, disulfide, mixed disulfide, thiosufinate or mixed thiosulfinate so as to cause thiol residues to become disulfide bonded to cysteines contained in the protein.
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Claims
WHAT IS CLAIMED IS: 1. A method of producing a comestible product to be ingested by a host for delivering a bioavailable thiol to the host, comprising: providing an ingestible material comprising a cyst (e) ine-containing protein; providing at least one compound selected from the group of thiols, disulfides, mixed disulfides, thiosufinates and mixed thiosulfinates; and treating said ingestible material with said at least one compound so as to cause thiol residues to become disulfide bonded to cysteines contained in said protein.
The method of claim 1 where said at least one compound comprises allyl mercaptan.
The method of claim 1 where said at least one compound comprises diallyl disulfide.
The method of claim 3 where said diallyl disulfide is a constituent of garlic oil.
The method of claim 1 where said at least one compound comprises allicin.
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The method of claim 1 wherein said ingestible material comprises a foodstuff.
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The method of claim 6 wherein said at least one compound is provided in a liquid and said treating step comprises mixing said liquid with said foodstuff.
The method of claim 6 wherein said at least one compound is provided in a liquid and said treating step comprises applying said liquid to said foodstuff so as to enable said at least one compound to permeate into said foodstuff .
The method of claim 6 wherein said at least one compound is provided in a liquid and said treating step comprises injecting said liquid into said foodstuff. 10. The method of claim 1 wherein said ingestible material comprises a dietary supplement.
The method of claim 10 wherein said at least one compound is provided in a liquid and said treating step comprises mixing said liquid with said dietary supplement.
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A comestible composition to be ingested by a host for delivering a bioavailable thiol to the host, comprising: an ingestible material comprising a cyst (e) ine-containing protein; wherein said ingestible material has been treated with at least one compound selected from the group of thiols, disulfides, mixed disulfides, thiosufinates and mixed thiosulfinates, so as to cause thiol residues to become disulfide bonded to cysteines contained in said protein.
The comestible composition of claim 12 , wherein said ingestible material is a foodstuff, and said foodstuff has been treated with allyl mercaptan so as to cause said thiol residues to become disulfide bonded to cysteines contained in said protein.
The comestible composition of claim 12, wherein said ingestible material is a foodstuff, and said foodstuff has been treated with diallyl disulfide so as to cause said thiol residues to become disulfide bonded to cysteines contained in said protein.
The comestible composition of claim 12 , wherein said ingestible material is a foodstuff, and said foodstuff has been treated with allicin so as to cause said thiol residues to become disulfide bonded to cysteines contained in said protein.
A nutraceutical or dietary supplement composition to be ingested by a host for delivering a bioavailable thiol to the host, comprising: a protein-containing substance containing thiol groups disulfide-bonded to one or more of the proteins of said substance, wherein said disulfide-bonded thiol groups are available to be metabolized in vivo by said host to allium- related organosulfur compounds selected from the group of thiols, disulfides, mixed disulfides, and thiosulfinates .
Protein bound S-AllylMercaptoCysteine of the formula: ProteinCyS-S-CH2-CH=CH2 where ProteinCyS represents a protein molecule that contains a cysteine.
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A compound to be administered to a host for delivering a bioavailable thiol to the host, comprising mercapto groups bound to a larger molecule such that the mercapto groups have low smell and taste prior to and during administration, said mercapto groups becoming liberated metabolically from said larger molecule to form thiols, disulfides, or mixed disulfides, said thiols, disulfides, or mixed disulfides being available for further transformation to thiosulfinates or mixed thiosulfinates when exposed to reactive oxygen species .
A compound to be administered to a host for delivering a bioavailable thiol to the host, comprising mercaptans non-covalently bound to a larger molecule such that the mercaptans have low smell and taste prior to and during administration, said mercaptans becoming liberated metabolically from said larger molecule to form thiols, disulfides, or mixed disulfides, said thiols, disulfides, or mixed disulfides being available for further transformation to thiosulfinates or mixed thiosulfinates when exposed to reactive oxygen species. 20. A compound administrable to a host, characterized in that said compound metabolizes to yield a disulfide or mixed disulfide capable of entering cells of said host, becoming reduced within said cells to at least one thiol capable of leaving said cells to the extracellular environment, said at least one thiol being capable of serving as an antioxidant in the extracellular environment and becoming oxidized therein to a disulfide or mixed disulfide capable of reentering said cells.